Multidimensional spectroscopies reveal a two-step process in a biomimetic supracomplex for oxygen evolution. A sub-ps charge-separation within the light-sensitizer moiety is followed by hole transfer from the catalyst counterpart, forming productive charges.
Tracking Ultrafast Charge Separation in a PBI-based Biomimetic Complex for Oxygen Evolution
Maiuri, Margherita;Russo, Mattia;Moretti, Luca;Cerullo, Giulio;
2020-01-01
Abstract
Multidimensional spectroscopies reveal a two-step process in a biomimetic supracomplex for oxygen evolution. A sub-ps charge-separation within the light-sensitizer moiety is followed by hole transfer from the catalyst counterpart, forming productive charges.File in questo prodotto:
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